Urban areas face challenges with water scarcity, and the use of non-conventional water resources for uses not requiring potable quality is being promoted more and more by governments and international agencies. However, non-conventional water resources, such as rainwater and greywater, need to be treated before use to avoid health risks and possible nuisance (smell, bacteria and algae proliferation in storage tanks, etc.). This study is aimed at demonstrating the feasibility of a system reusing treated greywater for toilet flushing, relying on a nature-based treatment technology—ground-based green façades—with limited maintenance requirements which is therefore easily replicable for decentralized treatment systems, like those of greywater reuse at building scales. The demonstrative system has been installed at the University of Jordan’s Al-Zahra dormitory in Amman and uses a degreaser as the primary treatment followed by ground-based green façade technology as a secondary treatment mechanism. The effluent is stored in an underground tank and directed to a tertiary treatment mechanism with UV lamps to remove pathogens before being reused for lawn irrigation and toilet flushing. Samples from influent and effluent were analyzed for various physical, chemical, and microbiological characteristics. The degreaser significantly reduced turbidity, TSS, total BOD5, and total COD levels in greywater. When combined with the green wall façades, the system demonstrated high removal efficiencies, particularly for turbidity, TSS, total COD, and total BOD5.